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Organozinc hydroxides, RZnOH, possessing the proton‐reactive alkylzinc group and the CO2‐reactive ZnOH group, represent an intriguing group of organometallic precursors for the synthesis of novel zinc carbonates. Comprehensive experimental and computational investigations on 1) solution and solid‐state behavior of tBuZnOH (1) species in the presence of Lewis bases, namely, THF and 4‐methylpyridine;...
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