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Li metal anodes are extensively studied owing to their unparalleled advantages in achieving high energy density. However, safety issues originating from dendritic Li growth are always a huge hindrance for applications in Li metal batteries (LMBs). In this study, a functional additive, 4,6‐dimethyl‐2‐mercaptopyrimidine (DMP), which is a typical leveler in the copper electroplating industry, is selected...