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Introduction of chirality into a supramolecular self‐assembly system plays an indispensable role in attaining specific molecular recognition ability. Herein, a chiral anticancer drug 5′‐deoxy‐5‐fluorouridine (5′DFU) was explored for inducing the self‐assembly of a cationic perylene diimide derivative containing boronic acid groups (PDI‐PBA) into a highly ordered right‐handed helical structure. As...
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