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Methan‐Oxidation In ihrer Zuschrift auf S. 18559 beschreiben J. Luo, Y. Li, Y. Wu et al., wie sich Ni‐Nanopartikel in einen N‐dotierten Kohlenstoffträger eingraben. Die Ni‐NPs lassen sich in Metalldefektzentren überführen, welche die C‐H‐Aktivierung in Methan katalysieren.
A surface digging effect of supported Ni NPs on an amorphous N‐doped carbon is described, during which the surface‐loaded Ni NPs would etch and sink into the underneath carbon support to prevent sintering. This process is driven by the strong coordination interaction between the surface Ni atoms and N‐rich defects. In the aim of activation of C−H bonds for methane oxidation, those sinking Ni NPs could...
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