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The synthesis of a class of electron‐rich amino‐functionalized β‐diketiminato (N‐nacnac) ligands is reported, with two synthetic methodologies having been developed for systems bearing backbone NMe2 or NEt2 groups and a range of N‐bound aryl substituents. In contrast to their (Nacnac)H counterparts, the structures of the protio‐ligands feature the bis(imine) tautomer and a backbone CH2 group. Direct...
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