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A biocatalyzed artificial photosynthesis system (APS) based on porphyrin/SiO2/Cp*Rh(bpy)Cl hybrid nanoparticles (TCPP/SiO2/Rh HNPs) to mimic chloroplasts in green plant is reported. The TCPP/SiO2/Rh HNPs are fabricated via sol–gel reaction of silica precursors functionalized with photosensitizer (porphyrin, TCPP) and electron mediator (Cp*Rh(bpy)Cl, M); while the integration of enzyme and coenzyme...
In article number 1705083, Jinjun Shi, Songping Zhang, and co‐workers present an integrated artificial photosynthesis system mimicking the structure and function of photosynthesis process performed by chloroplasts in green plants. Upon light irradiation, photo‐induced electrons transfer from a photosensitizer via an electron mediator to an oxidized coenzyme for its regeneration to NADH, which can...
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