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The thermally induced spin‐crossover (SCO) phenomenon in transition metal complexes is an entropy‐driven process, which has been extensively studied through calorimetric methods. Yet, the excess heat capacity associated with the molecular spin‐state switching has never been explored for practical applications. Herein, the thermal damping effect of an SCO film is experimentally assessed by monitoring...
Thin films of the molecular spin‐crossover complex [Fe(HB(1,2,4‐triazol‐1‐yl)3)2] undergo spin transition above room temperature, which can be exploited in sensors, actuators, and information processing devices. Variable temperature viscoelastic mapping of the films by atomic force microscopy reveals a pronounced decrease of the elastic modulus when going from the low spin (5.2 ± 0.4 GPa) to the high...
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