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In this work, it is demonstrated that random copolymerization is a simple but effective strategy to obtain new conductive copolymers as high‐performance thermoelectric materials. By using a polymerizing acceptor unit diketopyrropyrrole with donor units thienothiophene and oligo ethylene glycol substituted bithiophene (g32T), it is found that strong interchain donor–acceptor interactions ensure good...
A drop in carrier mobility at high doping levels dramatically hampers the improvement of thermoelectric performance of conductive polymers. In article number 2004378, Hui Li, Lidong Chen, and co‐workers propose a new strategy to synergistically improve carrier mobility and molecular doping by randomly copolymerizing donor‐acceptor type and donor‐donor type building blocks along a polymer backbone...
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