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The precise phase control of Cs‐Pb‐Br derivatives from 3D CsPbBr3 to 0D Cs4PbBr6 highly determines the photovoltaic performance of all‐inorganic CsPbBr3 perovskite solar cells (PSCs). Herein, the preferred phase conversion from precursor to Cs‐Pb‐Br derivatives is revealed by theoretically calculating the Gibbs free energies (∆G) of various phase conversion processes, allowing for a simplified multi‐step...
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