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Electrosynthesis of formic acid/formate is a promising alternative protocol to industrial processes. Herein, a pioneering pair‐electrosynthesis tactic is reported for exclusively producing formate via coupling selectively electrocatalytic methanol oxidation reaction (MOR) and CO2 reduction reaction (CO2RR), in which the electrode derived from Ni‐based metal–organic framework (Ni‐MOF) nanosheet arrays...
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