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Purple acid phosphatases (PAPs) are the only dinuclear metallohydrolases for which the necessity for a heterovalent active site (FeIII–MII; M = Fe, Zn or Mn) for catalysis has been established. A major goal for the synthesis of PAP biomimetics is to design a ligand in which the two coordination sites exhibit discrimination between the trivalent and divalent metal ions. With this goal in mind the ligand...
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