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Emerging multi‐resonance (MR) thermally activated delayed fluorescence (TADF) emitters can combine 100% exciton harvesting and high color purity for their organic light‐emitting diodes (OLED). However, the highly planar configurations of MR molecules lead to intermolecular‐interaction‐induced quenching. A feasible way is integrating host segments into MR molecules, namely a “self‐host” strategy, but...
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