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The achievement of excellent catalytic activity for electricity‐driven CO2 reduction over a wide potential window is significant for the mature applications. However, the efficient potential range is always limited by the dilemma in CO2 activation and product desorption at different potentials, due to the scaling relationships of adsorption energy. Herein, we developed a nanostructured Ag‐CO3 electrocatalyst...
The enhancement of catalytic activity is always limited by the dilemma in activation and desorption due to Sabatier principle. Locating the Sabatier optimum by manipulating catalyst electronic structure has been a long‐standing challenge in heterogeneous catalysis. Herein, we presented a generic strategy to continuously tailor the Pt 5d state occupancy via tuning the PtOMn electronic linkage over...
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