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A critical step in advancing the practical application of copper‐based organic light‐emitting diodes (OLEDs) is to bridge the large gap between device efficiency and operational stability at practical luminance. Described is a panel of air‐ and thermally stable two‐coordinate CuI emitters featuring bulky pyrazine‐ (PzIPr) or pyridine‐fused N‐heterocyclic carbene (PyIPr*) and carbazole (Cz) ligands...
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