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Hydrophobe Wassermoleküle wurden an der Grenzfläche zwischen einer Goldelektrode und einem wässrigen Elektrolyten mit Schwingungs‐Summenfrequenz‐Spektroskopie nachgewiesen. R. K. Campen et al. erklären in der Zuschrift auf S. 4275, dass die Populations‐ und Strukturmerkmale dieses Wassertyps von der Vorspannung abhängen. Sun Wukong, eine Gestalt der chinesischen Mythologie, schwingt seinen goldbebänderten...
Quantitative description of reaction mechanisms in aqueous phase electrochemistry requires experimental characterization of local water structure at the electrode/aqueous interface and its evolution with changing potential. Gaining such insight experimentally under electrochemical conditions is a formidable task. The potential‐dependent structure of a subpopulation of interfacial water with one OH...
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