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Overtone bands in the spectral range of 1300−1920 cm–1 have been found in Raman scattering spectrum of lithium tantalate single crystals. The Raman spectra were recorded in the 180° scattering geometry. The intensity of overtone transitions differs for different samples and, in some cases, is comparable with the Raman scattering intensity at the fundamental modes of a lithium tantalate single crystal.
— We have found conditions for high-speed measurements of Raman spectra of lithium niobate and lithium tantalate single crystals and ceramics. To measure Raman spectra, we used 180° scattering geometry and a minispectrometer equipped with an array detector. The Raman spectra obtained at two distinct orientations of the single crystals relative to the excitation beam direction have been shown to have...
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