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A synergic combination of a soluble redox mediator and a protected Li metal electrode to prevent the self‐discharge of the redox mediator is realized by exploiting a 2,2,6,6‐tetramethylpiperidinyl 1‐oxyl (TEMPO) redox mediator and an Al2O3/PVdF‐HFP composite protective layer (CPL). Stabilization of Li metal by simple CPL coating is effective at suppressing the chemical reduction of the oxidized...
As described on page 857, synergic combination of a soluble redox mediator and a protected lithium (Li) metal electrode is successfully demonstrated by J.‐K‐ Park, H.‐T. Kim, and co‐workers by exploiting a redox mediator of 2,2,6,6‐tetramethylpiperidinyl 1‐oxyl (TEMPO) and a composite protective layer (CPL). Self‐discharge, resulting from extensive migration and chemical reduction of the oxidized...
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