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Herein, efficient fabrication of polymersomes that have unique and nonequilibrium morphologies is reported. Starting from preparing big polymeric vesicles sized around 2 µm with a flexible but crosslinkable structure, a controllable morphological transformation process from the vesicles via prolate vesicles and the pearl‐chain‐like structure, which are the two intermediate structures, to vesicle‐end‐capped...
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