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The adjustment of the valence state of metal ions is crucial for various applications because peculiar activity originates from metal ions with specific valence. Cu+ can interact with molecules possessing unsaturated bonds like CO via π‐complexation, while Cu2+ doesn't have such ability. Meanwhile, Cu+ sites are easily oxidized to Cu2+, leading to the loss of activity. Despite great efforts, the development...
The dynamics rate of traditional metal carbides (TMCs) is relatively slow, severely limiting its fast‐charging capacity for lithium‐ion batteries (LIBs). Herein, the core–shell W@WxC heterostructure is developed to form Mott–Schottky heterostructure, thereby simultaneously accelerating the electronic and ionic transport kinetics during the charging/discharging process. The W nanoparticles are partially...
Lithium‐sulfur battery (LSB) is widely regarded as the most promising next‐generation energy storage system owing to its high theoretical capacity and low cost. However, the practical application of LSBs is mainly hampered by the low electronic conductivity of the sulfur cathode and the notorious “shuttle effect”, which lead to high voltage polarization, severe over‐charge behavior, and rapid capacity...
Photoresponsive covalent organic frameworks (PCOFs) have emerged as attractive candidates for adsorption, but it is challenging to construct PCOF adsorbents due to structural order loss of covalent organic frameworks (COFs) after introducing photoresponsive motifs and/or tedious steps of postmodification. Here, a facile strategy is developed, by dispersing photoresponsive metal‐organic polyhedra (PMOP)...
Recent research shows that the continuing importance of carbon anode materials plays an important role in the development of sodium‐ion batteries. Nevertheless, the practical deployment of sodium‐ion batteries still faces many challenges such as mediocre sodium storage capability and short cycle life. Therefore, it is imperative to explore improvement methods to boost their competitiveness. Herein,...
Benefiting from the natural abundance and low standard redox potential of potassium, potassium‐ion batteries (PIBs) are regarded as one of the most promising alternatives to lithium‐ion batteries for low‐cost energy storage. However, most PIB electrode materials suffer from sluggish thermodynamic kinetics and dramatic volume expansion during K+ (de)intercalation. Herein, it is reported on carbon‐coated...
Sodium‐ion batteries (NIBs) are an emerging technology, which can meet increasing demands for large‐scale energy storage. One of the most promising cathode material candidates for sodium‐ion batteries is Na3V2(PO4)3 due to its high capacity, thermal stability, and sodium (Na) Superionic Conductor 3D (NASICON)‐type framework. In this work, the authors have significantly improved electrochemical performance...
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