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Analogues of the [2Fe‐2S] subcluster of hydrogenase enzymes in which the central group of the three‐atom chain linker between the sulfur atoms is replaced by GeR2 and SnR2 groups are studied. The six‐membered FeSCECS rings in these complexes (E=Ge or Sn) adopt an unusual conformation with nearly co‐planar SCECS atoms perpendicular to the Fe‐Fe core. Computational modelling traces this result to the...
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