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The aggregation dependent correlation between fluorescence quenching and the electronic carotenoid–chlorophyll interactions, ϕCouplingCar S1-Chl, as measured by comparing chlorophyll fluorescence observed after two- and one-photon excitation, has been investigated using native LHC II samples as well as mutants lacking Chl 2 and Chl 13. For native LHC II the same linear correlation between ϕCouplingCar...
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