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Using a novel tricompartmental hydrazone ligand, a set of trinuclear Dy3 complexes has been isolated and structurally characterized. Complexes Dy3⋅ Cl, Dy3⋅ Br, and Dy3⋅ ClO4 feature a similar overall topology but different anions (Cl−, Br−, or ClO4−) in combination with exogenous OH− and solvent co‐ligands, which is found to translate into very different magnetic properties. Complex Dy3⋅ Cl shows...
Photosensitive lanthanide‐based single‐molecule magnets (Ln−SMM) are very attractive for their potential applications in information storage, switching, and sensors. However, the light‐driven structural transformation in Ln−SMMs hardly changes the coordination number of the lanthanide ion. Herein, for the first time it is reported that X‐ray (λ=0.71073 Å) irradiation can break the coordination bond...
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