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Direct copolymerization of olefin with polar monomers via a coordination‐insertion mechanism appears as the most efficient and attractive method to prepare functionalized polyolefins. Herein, we carried out direct copolymerization of ethylene and allyl acrylate by a bulky phosphino‐phenolate nickel catalyst, in which high‐molecular‐weight copolymers bearing polar five‐membered and six‐membered ring...
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