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The development of efficient electrocatalysts for the CO2 reduction reaction (CO2RR) remains a challenge. Demonstrated here is a NiSn atomic‐pair electrocatalyst (NiSn‐APC) on a hierarchical integrated electrode, which exhibits a synergistic effect in simultaneously promoting the activity and selectivity of the CO2RR to formate. The NiSn atomic pair consists of adjacent Ni and Sn, each coordinated...
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