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A landscape of mechanistic possibilities for the oxidation of olefins by bio-inspired non-heme iron catalysts has been explored in this work. The complexes studied consist of iron centers coordinated to the tetradentate N4 ligands tpa and bpmen, which provide two cis-labile sites to the iron center. These complexes catalyze conversion of olefin substrates into epoxide and/or cis-diol products. The...
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