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Emerging printed large‐area polymer light‐emitting diodes (PLEDs) are essential for manufacturing flat‐panel displays and solid lighting devices. However, it is challenging to obtain large‐area and stable ultradeep‐blue PLEDs because of the lack of light‐emitting conjugated polymers (LCPs) with robust deep‐blue emissions, excellent morphological stabilities, and high charging abilities. Here, a novel...