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The size of support in heterogeneous catalysts can strongly affect the catalytic property but is rarely explored in light‐driven catalysis. Herein, we demonstrate the size of TiO2 support governs the selectivity in photothermal CO2 hydrogenation by tuning the metal‐support interactions (MSI). Small‐size TiO2 loading nickel (Ni/TiO2‐25) with enhanced MSI promotes photo‐induced electrons of TiO2 migrating...
Strong metal‐support interactions (SMSI) have gained great attention in the heterogeneous catalysis field, but its negative role in regulating light‐induced electron transfer is rarely explored. Herein, we describe how SMSI significantly restrains the activity of Ru/TiO2 in light‐driven CO2 reduction by CH4 due to the photo‐induced transfer of electrons from TiO2 to Ru. In contrast, on suppression...
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