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Metallohydrogels are attractive biomaterials, whereas formation of a selective bimetallogel in aqueous solution has rarely been explored. In this study, we show that a phenylalanine derivative containing a 4‐pyridine group can not only assemble to form single crystals with copper acetate, but also selectively generate a Cu‐Ag bimetallohydrogel upon further addition of silver nitrate, which exhibits...
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