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Formation of a glue‐nanofiller layer between grains, consisting of a middle‐temperature spinel‐like LixCoO2 phase, reinforces the strength of the incoherent interfacial binding between anisotropically oriented grains by enhancing the face‐to‐face adhesion strength. The cathode treated with the glue‐layer exhibits steady cycling performance at both room‐temperature and 60 °C. These results represent...
The formation of a spinel LixCoO2 layer in a Ni‐rich secondary particle for lithium‐ion batteries is reported by S. K. Kwak, J. Cho, and co‐workers on page 4705, who find that the spinel‐like LixCoO2 layer, between layered primary particles, can enhance the mechanical strength of secondary particles by enhancing the interfacial binding energy among the grains. Moreover, the layer can effectively protect...
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