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Herein, we present a new class of singlet fission (SF) materials based on diradicaloids of carbene scaffolds, namely cyclic (alkyl)(amino)carbenes (CAACs). Our modular approach allows the tuning of two key SF criteria: the steric factor and the diradical character. In turn, we modified the energy landscapes of excited states in a systematic manner to accommodate the needs for SF. We report the first...
Die Verschränkung von Zuständen ist ein faszinierendes Resultat der Quantenphysik. Bei der Singulett‐Fission evolviert ein Paar von Chromophoren im S1S0‐Zustand in den spinverschränkten T1T1‐Zustand. Während sich die meisten Studien auf alternierende Kohlenwasserstoffe beschränken, ist das Potenzial von Diradikaloiden als Chromophore für die Singulett‐Fission weitgehend unerforscht. In ihrem Forschungsartikel...
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