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Tuning the electronic structure of metal–organic frameworks is the key to extending their functionality to the photocatalytic conversion of absorbed gases. Herein we discuss how the band edge positions in zeolitic imidazolate frameworks (ZIFs) can be tuned by mixing different imidazole‐based linkers within the same structure. We present the band alignment for a number of known and hypothetical Zn‐based...
Zeolithische Imidazolat‐Gerüste: R. Grau‐Crespo, S. Hamad et al. demonstrieren in ihrer Zuschrift auf S. 16246 ff., wie sich die Bandlücken und Bandkantenlagen in zeolithischen Imidazolat‐Gerüsten durch die Verwendung von Linkermischungen gezielt einstellen lassen.
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