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Visible‐light‐induced photoreaction of carboranes is an effective approach to prepare carborane‐containing compounds. While several methods involving boron‐centered carboranyl radicals have been established, those for carbon‐centered carboranyl radicals are underdeveloped, except for the UV‐light‐promoted photohomolysis. Herein, we describe a simple but effective approach to access carbon‐centered...
Carbon‐centered carboranyl radicals are an underdeveloped compound class. In their Research Article (e202305088), Zhi‐Xiang Wang, Xiang‐Yu Chen and co‐workers show that the combination of carborane phosphonium salts and KOAc forms a photoactive charge transfer complex for the generation of carbon‐centered carboranyl radicals, allowing access to various carborane‐oxindole pharmaceuticals.
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