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Ikarugamycin is a member of the polycyclic tetramate macrolactams (PTMs) family of natural products with diverse biological activities. The biochemical mechanisms for the formation of polycyclic ring systems in PTMs remain elusive. The enzymatic mechanism of constructing an inner five‐membered ring in ikarugamycin is reported. A three‐gene‐cassette ikaABC from the marine‐derived Streptomyces sp. ZJ306...
Der Biosyntheseweg von Himastatin aus Streptomyces himastatinicus wurde durch Genomanalyse, die Erzeugung von Gendeletionsmutanten und Komplementierungsexperimente aufgeklärt. Drei Cytochrome P450, die neuartige postmodifizierende Oxidationen katalysieren (siehe Bild), werden charakterisiert.
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