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Developing luminescent materials that exhibit strong emissions in both solution and solid phases is highly desirable and challenging. Herein, we report imine‐bond directed formation of a rigid organic cage (TPE‐cage) that was synthesized by [2+4] imine condensation of a TPE‐cored tetra‐aldehyde (TPE‐TA) with a clip‐like diamine (XA) to illustrate confinement‐induced fluorescence enhancement. Compared...
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