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Herein, the exposure of highly‐active nitrogen cation sites has been accomplished by photo‐driven quasi‐topological transformation of a 1,10‐phenanthroline‐5,6‐dione‐based covalent organic framework (COF), which contributes to hydrogen peroxide (H2O2) synthesis during the 2‐electron O2 photoreduction. The exposed nitrogen cation sites with photo‐enhanced Lewis acidity not only act as the electron‐transfer...
Herein, the exposure of highly‐active nitrogen cation sites has been accomplished by photo‐driven quasi‐topological transformation of a 1,10‐phenanthroline‐5,6‐dione‐based covalent organic framework (COF), which contributes to hydrogen peroxide (H2O2) synthesis during the 2‐electron O2 photoreduction. The exposed nitrogen cation sites with photo‐enhanced Lewis acidity not only act as the electron‐transfer...