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The trivalent ate complex [Cp*2CeCl2K(thf)] (Cp* = C5Me5) was used in a diverse set of salt metathesis reactions. Equimolar reactions with LiNiPr2, LiN(SiHMe2)2, KN(SiMe3)2, and LiCH2C6H4‐o‐NMe2 gave the alkali metal‐free complexes [Cp*2Ce(NiPr2)], [Cp*2Ce{N(SiHMe2)2}], [Cp*2Ce{N(SiMe3)2}], and [Cp*2Ce(CH2C6H4‐o‐NMe2)]. Employing [Cp*2CeCl2K(thf)] and KC≡CtBu in a 1:2 ratio produced a mixture of [Cp*...
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