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A photo-induced spin-flopping transition was observed below 5 K, lower than the Curie temperature (T c = 25 K), in a new charge-transfer-type magnet of manganese porphyrin derivative and tetracyanoethylene (TCNE). While the spin-flopping transition on interchain spin alignments takes place irreversibly in high external field, the transition is induced reversibly by the photoirradiation, depending...
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