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The improvement of molecular ordering in conducting polymers from disordered aqueous solution state to highly ordered solid state is investigated by K. Lee and co‐workers on page 8625. A well‐ordered structure, like a wall, can be formed by painting a mixture solution of PEDOT:PSS with an ionic liquid and then evaporating the water solvent. The different colors in the wall represent units of conducting...
The molecular ordering of aqueous conducting polymers is controlled using a rational method. By introducing various ionic liquids, which have designed electrostatic interactions to PEDOT:PSS solutions, the evolution of the molecular ordering of the PEDOT is manipulated. Consequently, highly ordered nanostructures are achieved with a reduced π–π stacking distance of ≈3.38 Å and, thus, a maximum σdc...
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