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A kinetic study on CH 4 combustion over a PdO/ZrO 2 (10%, w/w) catalyst has been performed in a temperature range between 400 and 550 o C by means of an annular catalytic microreactor.The role of mass transfer phenomena including diffusion in the catalyst pore, gas-solid diffusion and axial diffusion in the gas phase, has been preliminary addressed by means of mathematical...
The collection of chemical kinetics data in catalytic combustion over very active palladium catalysts under conditions relevant to practical applications (e.g. gas turbine combustors) is extremely difficult, mainly due to strong exothermicity and very fast rate of combustion reactions. Within this purpose in this paper two types of laboratory structured reactors, which closely resemble industrial...
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