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Dendritic growth and severe side reactions remain challenging problems for advancing aqueous zinc‐ion batteries. Those critical issues are closely related to the interfacial chemistry, solvation structure, and transportation kinetics of zinc ions. Herein, a regulated ion‐conductive electrode–electrolyte interface (PVA‐Zn(CF3SO3)2‐Si3N4, denoted as PZS) on Zn metal has been in situ constructed, which...
The Zn metal anode is considered one of the most promising anode choices for aqueous Zn‐based batteries. Nevertheless, dendrites and intricate side reactions have hindered its usage. Herein, an elastic and anti‐corrosive interlayer is introduced to address the problem. The idiosyncratic dielectric behavior of amorphous and nanostructured silicon nitride (Si3N4) is utilized to manipulate the ion kinetics,...
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