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Manipulation of long‐range order in 2D van der Waals (vdW) magnetic materials (e.g., CrI3, CrSiTe3 ,etc.), exfoliated in few‐atomic layer, can be achieved via application of electric field, mechanical‐constraint, interface engineering, or even by chemical substitution/doping. Usually, active surface oxidation due to the exposure in the ambient condition and hydrolysis in the presence of water/moisture...
Herein, the anisotropic magnetic properties of 2D van der Waals (vdW) insulator, chromium oxychloride (CrOCl), are presented. Temperature‐dependent bulk magnetization reveals a paramagnetic to antiferromagnetic phase transition at ≈14 K (Néel temperature, TN) while cooling. From the magnetic field‐dependent magnetization study (M–H) at low temperature, a first‐order field‐induced (at or above 40...
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