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Inspired by the recent experimental synthesis of graphene nanoribbons (GNRs) and theoretical research on their edge-decoration, we comprehensively studied the electrocatalytic performance of GNRs edge-decorated with Cu for CO2 reduction. Compared to zigzag GNRs, the Cu-terminated armchair GNRs with a width of n = 3p + 2 were more efficient catalysts for producing methanol from CO2 with a free energy...
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