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Cs2SnX6 (X = I, Br, and Cl), a vacancy‐ordered double perovskite, has recently emerged as a promising lead‐free perovskite for optoelectronic applications. The low quality of solution‐processed Cs2SnX6 perovskites, on the other hand, precludes further improvement of their performance in the devices. In this work, we developed a facile one‐step solution strategy for synthesizing high‐quality Cs2SnI...
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