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We present a spectroscopic investigation of the light-harvesting role of carotenoids in aggregates of the IsiA pigment–protein complex of the cyanobacterium Synechocystis PCC 6803. The results show that carotenoids in IsiA transfer energy on the sub-100fs timescale from the S 2 state to chlorophyll to about the same extent as in the related pigment–protein complexes CP43 and CP47. Selective...
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