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The thermodynamics of the Ti–Ni system are reviewed, and CALPHAD descriptions of metastable intermetallic phases are presented. These phases play an important role as precipitates in shape memory alloys. Metastable Ti3Ni4 and Ti2Ni3 are described as line compounds. Their thermodynamic model parameters are optimized with experimental solvus data and molar enthalpies at 0K from new first-principles...
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