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Sunlight‐driven photoreduction of the environmentally mobile uranyl (VI) to less soluble tetravalent uranium is of considerable value to environmental sustainability, yet the pursuit for high‐performance semiconductors is plagued by the current disadvantages of inferior charge separation/migration. This study reports that a nickel single atom isolated on a sulfur‐functionalized graphitic carbon nitride/reduced...
Coupling the photoproduction of solar fuel and value‐added chemicals is highly attractive, as it maximizes the utilization of incident sunlight and the economic value of photocatalytic reactions. Constructing intimate semiconductor heterojunction for these reactions is highly desirable due to accelerated charge separation at the interfacial contact, but is challenged by material synthesis. Here, an...