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A new reforming process was studied using Ni/SiO2 with a hydrogen-permeating membrane reactor. Nickel catalyst supported on SiO2 is highly active for CH4−H2O−O2 reaction in membrane reactor and the reaction close to CH4+0.35O2+1.3H2O→CO2+3.3H2 proceeds at 873 K. Since the selectivity to carbon and CO2 increased and decreased with decreasing contact time respectively, it is considered that the reaction...
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