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The spin Hamiltonian parameters (SHPs) (i.e., g factors, hyperfine structure constants and superhyperfine parameters) are theoretically investigated for the irradiation induced Rh2+ and Rh0 centres in NH4Cl by use of the perturbation calculations. The tetragonally compressed Rh2+ centre in the form of [RhCl4(H2O)2]2‾ group originates from interstitial Rh2+ (reduced from original Rh3+ of doped RhCl...
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