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Herein, highly efficient composite photocatalysts comprising black Cu-doped TiO2 nanoparticles (BCT) encapsulated within hierarchical flower-like NiAl-layered double hydroxide (LDH) microspheres were fabricated via a one-step hydrothermal route. Cu-doping and subsequent reduction treatment led to extended visible-light absorption of TiO2 in the resulting composites, as confirmed by ultraviolet-visible...
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