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A robust self‐assembly of nanoparticles into fibers and 3D scaffolds is designed and fabricated by functionalizing a RAFT‐polymerized amphiphilic triblock copolymer with designer ionic complementary peptides so that the assembled core–shell polymeric nanoparticles are directed by peptide assembly into continuous “nanoparticle fibers,” ultimately leading to 3D fiber scaffolds. The assembled nanostructure...
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